Observation of the triplet exciton in EuS-coated single-walled nanotubes.

Title Observation of exciton-phonon sideband in individual metallic single-walled carbon nanotubes

Direct experimental evidence of exciton-phonon bound states in carbon nanotubes.

We present direct experimental observation of exciton-phonon bound states in the photoluminescence excitation spectra of isolated single-walled carbon nanotubes (SWNT) in aqueous suspension. The photoluminescence excitation spectra from several distinct SWNTs show the presence of at least one sideband related to the tangential modes, lying 0.2 eV above the main absorption or emission peak. Both...

Observation of exciton-phonon sideband in individual metallic single-walled carbon nanotubes.

Single-walled carbon nanotubes (SWCNTs) are quasi-one-dimensional systems with poor Coulomb screening and enhanced electron-phonon interaction, and are good candidates for excitons and exciton-phonon couplings in metallic state. Here we report backscattering reflection experiments on individual metallic SWCNTs. An exciton-phonon sideband separated by 0.19 eV from the first optical transition pe...

Multiple exciton generation by a single photon in single-walled carbon nanotubes.

Multiple-exciton generation in single-walled carbon nanotubes is investigated theoretically. We show that multiple excitons can be directly generated by a single photon through resonant coupling with multiexciton states. Further, the theoretically predicted threshold energy for this process is consistent with recent experimental results. Our calculations clarify the elementary processes of mult...

Suppression of exciton-electron scattering in doped single-walled carbon nanotubes.

We theoretically study the phase relaxation of excitons in doped single-walled carbon nanotubes caused by elastic scattering between an exciton and an electron. Our calculation of the spectral linewidth, that is the inverse of the scattering rate, demonstrates that this dephasing process is unexpectedly suppressed in doped single-walled carbon nanotubes, giving rise to anomalous nonlinear behav...